If the number is already in your call history (either as dialled or received. Not as message history), then just select 'Add to reject list' at the bottom of the screen and then select the number you wish to block. If its not in call history, just dial the number and cut the call. Then follow the above steps.
Why not try LEO Privacy? There is a funcrion which name Harassment Interception, you can use this applock to block certain unwanted calls, this is very helpful for me. Hope this applock can also help you. LEO Privacy Applock Hide Safe Android Apps on Google Play
LEO Privacy can help you to block all spam and unwanted calls and lock all private apps. I suggest everyone to download it and check it out its feature.
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