You should just be able to plug the remote into your computer with the USB cable supplied, go to the Harmony website listed with your product packaging, and Harmony will walk you through (very user friendly interface) a process which sets up your personal account, downloads the necessary setup software into your remote, and automatically programs your remote to whatever device you identify. With what you've said, all you need in addition to the Samsung brand name is the model number. The rest is done by Harmony including code installations.
I have the Harmony 600, linked to a tv and vcr and the setup/programming process was as uncomplicated as anything I've seen.
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