You can delete music manually within Music app in iPod. Or you can try the 3rd-party tool Leawo iTransfer to delete music in batch with simple steps. Just follow the below instruction.
Download and install Leawo iTransfer on your computer. The below guide shows you how to delete music files from iTunes with iTransfer in detail.
Step 1: Connect your iPhone to computer
Connect your iPhone to computer and then launch Leawo iTransfer. It will detect your iPhone instantly.
Step 2: Choose music to delete on iPhone for iTunes
Open your iPhone's Library and then go to Music tab to choose the songs you want to delete from iTunes. Just tick the ones you don't want.
Step 3: Delete songs
On the upper side, you could see a "Delete" option, by clicking which you could then freely delete songs you don't want. Confirm the music deletion by clicking "Yes" on the pop-up "Delete Media" interface.
After deleting songs from iPhone, you could then sync your songs to iTunes. If you have logged in iTunes with the Apple ID you have logged on your iPhone, the result will by synced easily.
For more details, check: How to Delete Music from iTunes
To delete music from your ipod you must delete it from itunes
connect the usb cord that connects your ipod and computer. open your itunes go to your music files right click to the song(s) you want to delete once you completed this steps SYNC your ipod. uplug your ipod this should help
SOURCE: downloading music from my computer,deleting music
For an Ipod you basically NEED to use Itunes. If you have trouble with anything, just click on support.
http://www.apple.com/itunes/
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