See if this helps you out..
To resolve this you need to alter the port that your iPhone or iPad uses to send mailwhich can be done as follows. Go to Mail, Contacts, Calendars and select the account you wish to change. On the next screen, scroll down to the "Outgoing Mail Server" section and select the SMTP server that is listed.
Why can't I send mail from my iPhone or iPad? - Knowledgebase ...
customer.maginternet.co.uk/.../65/Why-cant-I-send-mail-from-my-iPhone-or-iPad.html
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