There is a sync button next to the Play and Charge port on the controller, all you have to do is press both the sync button on the Xbox and the controller and it should connect.
On the nonslim Xbox 360's the sync button is right next to the infared sensor and the memory card slots.
On the slim Xbox 360 the sync button will be right next to the usb ports on the front of the Xbox 360 console.
When you successfully start the sync the led's for the controller's and console's lights will spin and be ready for you to press the sync button on the other device.
(PS, you have to have both the console and the controller on for this to work; PPS, By controller on I mean having it searching)
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